Synthesis and Structure of a 1,2,4,5-Tetraborinane

Author:

Fisch Herbert,Pritzkow Hans,Siebert Walter

Publisher

Wiley

Subject

General Chemistry,Catalysis

Reference9 articles.

1. in : Boron Hydride Chemistry, Academic Press, New York 1975.

2. Boron-fluorine chemistry. II. Reaction of boron monofluoride with acetylenes

3. Classical configurations associated with nonclassical molecules: three carboranes as examples

4. Procedure: 2: A solution of Me3Si- NMe2 (7.9 g, 67.5 mmol) in pentane (35 mL) is added dropwise to a solution of (Cl2B)2CH2 [5] (6.0 g, 33.8 mmol) in pentane (35 mL). The mixture is heated under reflux for 2.5 h and then distilled at 25°C/0.01 torr. 1 is obtained in 84% yield (5.5 g). A solution of 1 (4.0 g, 20.6 mmol) in pentane (40 mL) is added to the Na/K alloy prepared from 1.44 g (37 mmol) K and 0.1 g (4.3 mmol) Na. During the ensuing reaction the mixture turns blue. After three days' stirring at 20°C the mixture is filtered. Distillation of the filtrate at 65°C/0.01 torr affords 2, which is recrystallized from CH2Cl2 (0.73 g, 29%; m.p. 144°C, decomp.).

5. Tris(dichloroboryl)methane, bis(dichlororyl)methane, and a possible new route to carbonarnes

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1. Triaminotriborane(3): A Homocatenated Boron Chain Connected by B−B Multiple Bonds;Angewandte Chemie International Edition;2017-11-02

2. Triaminotriborane(3): A Homocatenated Boron Chain Connected by B−B Multiple Bonds;Angewandte Chemie;2017-11-02

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