Toward High‐Throughput Single‐Spin Optically Detected Magnetic Resonance Spectroscopy with Spatially Programmable Laser Illumination

Author:

Cai Mingcheng1,Guo Zhongzhi1,Li Chunxing1,Li Simin2,Shi Fazhan13ORCID,Wang Mengqi1,Li Hui4,Wang Pengfei13ORCID,Du Jiangfeng13ORCID

Affiliation:

1. CAS Key Laboratory of Microscale Magnetic Resonance and School of Physical Sciences University of Science and Technology of China CAS Center for Excellence in Quantum Information and Quantum Physics University of Science and Technology of China Hefei 230026 P. R. China

2. College of Chemistry, Chemical Engineering and Materials Science Shandong Normal University Jinan 250014 P. R. China

3. Hefei National Laboratory University of Science and Technology of China Hefei 230088 P. R. China

4. Suzhou Institute of Biomedical Engineering and Technology Chinese Academy of Sciences Suzhou Jiangsu 215163 P. R. China

Abstract

AbstractThe single nitrogen‐vacancy (NV) centers in diamond are shown as a quantum sensor with broad applications in nanoscale sensing of magnetic field, electric field, temperature, and strain. However, the basic technique, namely, optically detected magnetic resonance to manipulate and measure single NV centers needs to be highly sped up for broad and practical applications. Here, this work shows a parallel optically detected magnetic resonance (ODMR) platform of single NV centers including the programmable excitation laser spots generated by a digital micromirror device, a four‐channel uniform microwave delivery, and the fluorescence detector based on scientific complementary metal–oxide–semiconductor camera. In the viewing field of 26 µm, hundreds of distinguishable fluorescent spots are addressed and 413 NV center spots are recognized. The magnetic resonance spectrum, Rabi oscillation, and spin echo of each NV center spot are measured in parallel. As a result, a preliminary speedup of ≈20‐fold is achieved compared to the confocal‐based ODMR and can be further extended to thousands of folds after updating the digital micromirror device and camera.

Funder

Chinese Academy of Sciences

National Natural Science Foundation of China

Publisher

Wiley

Subject

Electrical and Electronic Engineering,Computational Theory and Mathematics,Condensed Matter Physics,Mathematical Physics,Nuclear and High Energy Physics,Electronic, Optical and Magnetic Materials,Statistical and Nonlinear Physics

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