Light‐Driven MXene‐Based Microrobots: Mineralization of Bisphenol A to CO2 and H2O

Author:

Dekanovsky Lukas1,Huang Hai2,Akir Sana1,Ying Yulong2ORCID,Sofer Zdenek1ORCID,Khezri Bahareh134ORCID

Affiliation:

1. Department of Inorganic Chemistry University of Chemistry and Technology Prague Technická 5, Praha 6 16822 Prague Czech Republic

2. School of Materials Science and Engineering Zhejiang Sci‐Tech University Hangzhou 310018 P. R. China

3. Institute of Chemical Research of Catalonia (ICIQ) The Barcelona Institute of Science and Technology (BIST) Av. Països Catalans, 16 Tarragona E‐43007 Spain

4. Departament de Química Física i Inorgànica Universitat Rovira i Virgili C/Marcel·lí Domingo 1 Tarragona 43007 Spain

Abstract

AbstractLight‐driven magnetic MXene‐based microrobots (MXeBOTs) have been developed as an active motile platform for efficiently removing and degrading bisphenol A (BPA). Light‐driven MXeBOTs are facilitated with the second control engine, i.e., embedded Fe2O3 nanoparticles (NPs) for magnetic propulsion. The grafted bismuth NPs act as cocatalysts. The effect of the BPA concentration and the chemical composition of the swimming environment on the stability and reusability of the MXeBOTs are studied. The MAXBOTs, a developed motile water remediation platform, demonstrate the ability to remove/degrade approximately 60% of BPA within just 10 min and achieve near‐complete removal/degradation (≈100%) within 1 h. Above 86% of BPA is mineralized within 1 h. The photocatalytic degradation of BPA using Bi/Fe/MXeBOTs demonstrates a significant advantage in the mineralization of BPA to CO2 and H2O.

Funder

National Natural Science Foundation of China

Publisher

Wiley

Subject

General Materials Science,General Chemistry

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