Integrated Textile Supercapacitors Enhanced with Energy‐Absorbing Spacer Fabrics and Ti3C2Tx MXene

Author:

Zhang Peng1,Wang Zhiyu1,Zhang Hongjie2,Usman Ken Aldren1,Hegh Dylan1,Chen Shasha1,Yang Fangli13,Zhong Zhili4,Naebe Maryam1,Wang Xungai5,Qin Si1ORCID,Razal Joselito M.1ORCID

Affiliation:

1. Institute for Frontier Materials Geelong Waurn Ponds Campus Deakin University 75 Pigdons Road Waurn Ponds Victoria 3216 Australia

2. College of Textiles and Apparel Quanzhou Normal University Quanzhou Fujian 362000 China

3. School of Chemistry and Chemical Engineering Zhoukou Normal University Zhoukou 466000 China

4. Key Laboratory of Advanced Textiles Composites of Ministry of Education School of Textiles Science and Engineering Tiangong University Tianjin China

5. Research Centre of Textiles for Future Fashion JC STEM Lab of Sustainable Fibers and Textiles School of Fashion and Textiles The Hong Kong Polytechnic University Kowloon 999077 Hong Kong

Abstract

AbstractThe rapid development of wearable electronics requires energy storage devices capable of withstanding both static and dynamic deformations. The versatility of textile supercapacitors renders them promising candidates, but their low electrochemical performance especially under mechanical deformation, poses many limitations for practical use. In this study, MXene‐based textile supercapacitors are designed and fabricated using hierarchical spacer fabrics as the skeleton to provide robust mechanical support and stable performance. Ti3C2Tx MXene is adopted as the current collector and active material for the spacer fabric supercapacitor, resulting in an impressive areal capacitance of 415 mF cm−2 with a MXene loading of 4.2 mg cm−2. Remarkable stability and durability are achieved in the form of three‐dimensional (3D) textile supercapacitors, even under both static and dynamic deformations. The compressive behaviors of these supercapacitors can be easily adjusted (e.g., from 10 to 168 KPa at 50% compression) by altering the spacer fabric structure, demonstrating their energy‐absorption (damping of kinetic energy) capability and their potential to meet the requirements of various wearable applications.

Funder

Australian Research Council

Publisher

Wiley

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