Recent Advances in Hydrogenation of CO2 to CO with Heterogeneous Catalysts Through the RWGS Reaction

Author:

Zhang Wenting12,Sun Jiashu12,Wang Hongli1,Cui Xinjiang1ORCID

Affiliation:

1. State Key Laboratory for Oxo Synthesis and Selective Oxidation Lanzhou Institute of Chemical Physics Chinese Academy of Sciences No. 18, Tianshui Middle Road Lanzhou 730000 People's Republic of China

2. University of Chinese Academy of Sciences No. 19A, Yuquanlu Beijing 100049 People's Republic of China

Abstract

AbstractWith the continuous increase in CO2 emissions, primarily from the combustion of coal and oil, the ecosystem faces a significant threat. Therefore, as an effective method to minimize the issue, the Reverse Water Gas Shift (RWGS) reaction which converts CO2 towards CO attracts much attention, is an environmentally‐friendly method to mitigate climate change and lessen dependence on fossil fuels. Nevertheless, the inherent thermodynamic stability and kinetic inertness of CO2 is a big challenge under mild conditions. In addition, it remains another fundamental challenge in RWGS reaction owing to CO selectivity issue caused by CO2 further hydrogenation towards CH4. Up till now, a series of catalysis systems have been developed for CO2 reduction reaction to produce CO. Herein, the research progress of the well‐performed heterogeneous catalysts for the RWGS reaction were summarized, including the catalyst design, catalytic performance and reaction mechanism. This review will provide insights into efficient utilization of CO2 and promote the development of RWGS reaction.

Funder

National Natural Science Foundation of China

Publisher

Wiley

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