Unleashing the Potential of MXene‐Based Flexible Materials for High‐Performance Energy Storage Devices

Author:

Zhou Yunlei12ORCID,Yin Liting3,Xiang Shuangfei4,Yu Sheng5,Johnson Hannah M.5,Wang Shaolei6,Yin Junyi6,Zhao Jie7,Luo Yang89ORCID,Chu Paul K.9ORCID

Affiliation:

1. Hangzhou Institute of Technology Xidian University Hangzhou 311200 China

2. School of Mechano‐Electronic Engineering Xidian University Xi'an 710071 China

3. Department of Aerospace and Mechanical Engineering University of Southern California Los Angeles CA 90089 USA

4. School of Materials Science and Engineering and Institute of Smart Fiber Materials Zhejiang Sci‐Tech University Hangzhou 310018 China

5. Department of Chemistry Washington State University Pullman WA 99164 USA

6. Department of Bioengineering University of California Los Angeles Los Angeles CA 90095 USA

7. Molecular Engineering of Polymers Department of Material Science Fudan University Shanghai 200438 China

8. Department of Materials ETH Zurich Zurich 8093 Switzerland

9. Department of Physics Department of Materials Science and Engineering and Department of Biomedical Engineering City University of Hong Kong Kowloon Hong Kong 999077 China

Abstract

AbstractSince the initial discovery of Ti3C2 a decade ago, there has been a significant surge of interest in 2D MXenes and MXene‐based composites. This can be attributed to the remarkable intrinsic properties exhibited by MXenes, including metallic conductivity, abundant functional groups, unique layered microstructure, and the ability to control interlayer spacing. These properties contribute to the exceptional electrical and mechanical performance of MXenes, rendering them highly suitable for implementation as candidate materials in flexible and wearable energy storage devices. Recently, a substantial number of novel research has been dedicated to exploring MXene‐based flexible materials with diverse functionalities and specifically designed structures, aiming to enhance the efficiency of energy storage systems. In this review, a comprehensive overview of the synthesis and fabrication strategies employed in the development of these diverse MXene‐based materials is provided. Furthermore, an in‐depth analysis of the energy storage applications exhibited by these innovative flexible materials, encompassing supercapacitors, Li‐ion batteries, Li–S batteries, and other potential avenues, is conducted. In addition to presenting the current state of the field, the challenges encountered in the implementation of MXene‐based flexible materials are also highlighted and insights are provided into future research directions and prospects.

Funder

National Natural Science Foundation of China

Publisher

Wiley

Subject

General Physics and Astronomy,General Engineering,Biochemistry, Genetics and Molecular Biology (miscellaneous),General Materials Science,General Chemical Engineering,Medicine (miscellaneous)

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