Functional PDMS Elastomers: Bulk Composites, Surface Engineering, and Precision Fabrication

Author:

Li Shaopeng1,Zhang Jiaqi1,He Jian2,Liu Weiping13,Wang YuHuang45ORCID,Huang Zhongjie1ORCID,Pang Huan6ORCID,Chen Yiwang7

Affiliation:

1. State Key Laboratory for Modification of Chemical Fibers and Polymer Materials College of Materials Science and Engineering Donghua University Shanghai 201620 China

2. Yizhi Technology (Shanghai) Co., Ltd No. 99 Danba Road, Putuo District Shanghai 200062 China

3. Center for Composites COMAC Shanghai Aircraft Manufacturing Co. Ltd Shanghai 201620 China

4. Department of Chemistry and Biochemistry University of Maryland College Park MD 20742 USA

5. Maryland NanoCenter University of Maryland College Park MD 20742 USA

6. School of Chemistry and Chemical Engineering Yangzhou University Yangzhou Jiangsu 225009 China

7. National Engineering Research Center for Carbohydrate Synthesis/Key Lab of Fluorine and Silicon for Energy Materials and Chemistry of Ministry of Education Jiangxi Normal University 99 Ziyang Avenue Nanchang 330022 China

Abstract

AbstractPolydimethylsiloxane (PDMS)—the simplest and most common silicone compound—exemplifies the central characteristics of its class and has attracted tremendous research attention. The development of PDMS‐based materials is a vivid reflection of the modern industry. In recent years, PDMS has stood out as the material of choice for various emerging technologies. The rapid improvement in bulk modification strategies and multifunctional surfaces has enabled a whole new generation of PDMS‐based materials and devices, facilitating, and even transforming enormous applications, including flexible electronics, superwetting surfaces, soft actuators, wearable and implantable sensors, biomedicals, and autonomous robotics. This paper reviews the latest advances in the field of PDMS‐based functional materials, with a focus on the added functionality and their use as programmable materials for smart devices. Recent breakthroughs regarding instant crosslinking and additive manufacturing are featured, and exciting opportunities for future research are highlighted. This review provides a quick entrance to this rapidly evolving field and will help guide the rational design of next‐generation soft materials and devices.

Funder

National Natural Science Foundation of China

Natural Science Foundation of Shanghai Municipality

State Key Laboratory for Modification of Chemical Fibers and Polymer Materials

National Science Foundation

Publisher

Wiley

Subject

General Physics and Astronomy,General Engineering,Biochemistry, Genetics and Molecular Biology (miscellaneous),General Materials Science,General Chemical Engineering,Medicine (miscellaneous)

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