Oxide Solid–Solution Catalysts with Good Redox Properties for Liquid–Phase Aerobic Additive–Free Oxidation: A Review

Author:

Tada Shohei1ORCID,Kondo Masaru2ORCID,Joutsuka Tatsuya3ORCID

Affiliation:

1. Division of Applied Chemistry Hokkaido University N13W8, Kita-ku, Sapporo Hokkaido 060-8628 Japan

2. School of Pharmaceutical Sciences University of Shizuoka, Shizuoka Shizuoka 422-8526 Japan

3. Department of Materials Science and Engineering Ehime University, 3 Bunkyo-cho, Matsuyama Ehime 790-8577 Japan

Abstract

AbstractIn this review, we discuss liquid–phase redox reactions using oxide solid–solution catalysts. These oxide solid solutions are readily prepared by introducing various elements into the foundational metal oxide template. Doping with metal species leads to the formation of [MOx] clusters with unique coordination structures, which is a remarkable feature that deserves attention. Consequently, oxide solid solutions exhibit catalytic capabilities that extend beyond those of conventional metal–oxide catalysts. Notably, these [MOx] clusters occasionally exhibit exceptional redox activities that can be used to catalyze liquid–phase redox reactions. Hence, we conjecture that a connection exists between catalyst structure and activity. This review delves into oxide solid–solution catalysts through the lenses of organic chemistry, solid catalysts, and computational chemistry, thereby collectively shaping our understanding and prospects in this field.

Funder

Environmental Restoration and Conservation Agency

Ministry of the Environment, Government of Japan

Publisher

Wiley

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