Ring‐Opening Intramolecular Arylation of 1,2‐Disubtituted Epoxides with Tuneable Stereoselectivity-Reference-Cited by-同舟云学术

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Ring‐Opening Intramolecular Arylation of 1,2‐Disubtituted Epoxides with Tuneable Stereoselectivity

Published:2024-02-21 Issue:9 Volume:27 Page:
ISSN:1434-193X
Container-title:European Journal of Organic Chemistry
language:en
Short-container-title:Eur J Org Chem

Author:

Zhao Cong‐Cong¹²,Shen Chaoren²,Wang Bin²,Rong Liangce¹,Dong Kaiwu²^ORCID

Affiliation:

1. Jiangsu Key Laboratory of Green Synthetic Chemistry for Functional Materials School of Chemistry and Materials Science Jiangsu Normal University Xuzhou Jiangsu 221116 P. R. China

2. Shanghai Key Laboratory of Green Chemistry and Chemical Processes State Key Laboratory of Petroleum Molecular & Process Engineering School of Chemistry and Molecular Engineering East China Normal University Shanghai 200062 P. R. China

Abstract

AbstractA method of stereodivergent intramolecular ring‐opening arylation of amine‐tethered epoxides to 3,4‐disubstituted tetrahydroquinolines has been developed. The tuneable good stereoselectivity was attained by changing the catalyst from titanocene(III) catalyst to Lewis‐acidic zinc catalyst.

Funder

National Natural Science Foundation of China

Publisher

Wiley

Reference41 articles.

1. Stereodivergent Catalysis

2. Stereodivergent routes in organic synthesis: carbohydrates, amino acids, alkaloids and terpenes

3. New advances in dual stereocontrol for asymmetric reactions

4. Reversal of enantioselectivity in chiral metal complex-catalyzed asymmetric reactions

5. Recent topics of the stereodivergent synthesis of natural products

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