Mixing screw design and high density polyethylene toughening modification for recycled polypropylene based on screw 3D printing

Abstract

AbstractThe recycling of waste plastics primarily involves physical modification and the addition of modifiers, often utilizing equipment such as twin‐screw extruders for miscible modification. Considering the widespread use of single‐screw 3D printing, improving the mixing efficiency of the single‐screw is crucial to achieve a “one‐stop” recycling modification that is suitable for 3D printing. This paper introduces a 3D printer equipped with a mixing screw (MS) and compares it with a conventional screw (CS). We conduct numerical simulations to investigate the pressure build‐up capacity, velocity streamline distribution, and the mixing effect of the MS. The mechanical properties, thermal characteristics, and molecular orientation of the recycled Polypropylene (rPP) and high density polyethylene (HDPE) mixture are investigated through experiments. The results show that the MS provides more effective elongational flows compared to the CS by breaking down the reinforcing materials into smaller particles. Additionally, toughening and modification experiments are performed on rPP and HDPE. The composites treated with the MS showed improved elongation at break (increased by ~111%), a stable melt crystallization temperature, and an enhanced mixing effect. This study on single‐screw 3D printers lays the groundwork for streamlining the plastic recycling process and increasing the reuse rate of recycled plastics.