Facile Formation of Metal–Oxide Nanocraters by Laser Irradiation for Highly Enhanced Detection of Volatile Organic Compounds

Author:

Suh Jun Min1ORCID,Song Young Geun2,Seo Jung Hwan3,Noh Myoung Sub2,Kang Min Gyu4,Sohn Woonbae1,Lee Jinho5,Lee Kwangjae6,Cho Donghwi7,Jeon Seokwoo8,Kang Chong-Yun2,Shim Young-Seok9,Jang Ho Won110ORCID

Affiliation:

1. Department of Materials Science and Engineering Research Institute of Advanced Materials Seoul National University Seoul 08826 Republic of Korea

2. Center for Electronic Materials Korea Institutes of Science and Technology (KIST) Seoul 02791 Republic of Korea

3. Department of Mechanical & System Design Engineering Hongik University Seoul 04066 Republic of Korea

4. Department of Materials Science and Engineering Pennsylvania State University University Park PA 16802 USA

5. Department of Materials Science and Engineering KAIST Institute for the Nanocentury Korea Advanced Institute of Science and Technology (KAIST) Daejeon 34141 Republic of Korea

6. Department of Information Security Engineering Sangmyung University Cheonan 31066 Republic of Korea

7. Advanced Materials Division Korea Research Institute of Chemical Technology Daejeon 34114 Republic of Korea

8. Department of Materials Science and Engineering Korea University Seoul 02841 Republic of Korea

9. School of Energy, Materials and Chemical Engineering Korea University of Technology and Education Cheonan 31253 Republic of Korea

10. Advanced Institute of Convergence Technology Seoul National University Suwon 16229 Republic of Korea

Abstract

Although various fabrication methods for metal–oxide nanostructures have been well developed for enlarged surface area, numerous efforts to further enhance the effective surface area for their chemical sensor applications are still being studied. Herein, a high‐power laser is irradiated on the existing metal–oxide nanostructures to expose the hidden inner surface of the nanostructures for full participation in the surface gas‐sensing reactions, resulting in extraordinary gas‐sensing performance. In addition, noble metal catalyst decoration at both the inner and outer surfaces of the nanostructures records extremely high gas response and selectivity to volatile organic compounds. The numerical simulation and experimental verification of the effects of high‐power laser irradiation for morphological evolution of the metal–oxide nanostructures can provide a new perspective toward the time‐efficient development of nanostructure‐based electronic devices.

Publisher

Wiley

Subject

General Earth and Planetary Sciences,General Environmental Science

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