Asymmetric Additive‐Assisted Organic Solar Cells with Much Better Energy Harvesting and Wireless Communication Performance

Author:

Lei Wen1ORCID,Wang Yufei1,Liang Zezhou2,Feng Junyi3,Zhang Wei3,Fang Junbin1,Chen Zhe1,Hou Lintao1ORCID

Affiliation:

1. Guangdong Provincial Key Laboratory of Optical Fiber Sensing and Communications Guangdong Engineering Technology Research Center for Visible Light Communication Guangzhou Key Laboratory of Vacuum Coating Technologies and New Energy Materials Jinan University Guangzhou 510632 P. R. China

2. Key Laboratory for Physical Electronics and Devices of the Ministry of Education & Shaanxi Key Lab of Photonic Technique for Information School of Electronics Science & Engineering Faculty of Electronic and Information Engineering Xi'an Jiaotong University Xi'an 710049 P. R. China

3. School of Physics and Materials Science Guangzhou University Guangzhou 510006 P. R. China

Abstract

AbstractOrganic solar cells (OSCs), exhibiting better sensitivity to different light intensities and higher power conversion efficiencies (PCEs) under indoor illumination, have great potential to be simultaneously used for solar energy harvesting and optical communication. However, the poor intrinsic molecular stacking and phase separation in active layers significantly hinder the charge transport and extraction in OSCs for achieving this aim. Here, an effective heterohalogen‐substitution asymmetric additive strategy is proposed to fine‐tune the non‐covalent interaction with nonfullerene molecules and optimize the morphology of active layer, which greatly boosts both the OSC photovoltaic performance with the PCEs of up to 18.30% and 29.52% under AM 1.5G and indoor light illumination respectively, and the ‒3 dB communication bandwidths of 4.11, 3.14, and 3.04 MHz at red, green, and blue (RGB) wavelengths respectively. Of particular note, combining the wavelength division multiplexing and adaptive bit‐loading technologies, the visible light communication system comprised of the RGB light sources and additive‐treated OSCs delivers more remarkable data throughput of 302.7 Mb s−1 and higher harvesting power of 7.38 mW simultaneously, presenting an excellent self‐powered capability for enhanced endurance. This work demonstrates that high‐performance OSCs with excellent energy harvesting and wireless communication capacity can be perfectly achieved by a heterohalogen‐substitution asymmetric additive strategy.

Funder

National Natural Science Foundation of China

National Key Research and Development Program of China

Natural Science Foundation of Guangdong Province

Publisher

Wiley

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment

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