Multi‐Dimensional Characterization of Battery Materials

Author:

Ziesche Ralf F.1234ORCID,Heenan Thomas M. M.12ORCID,Kumari Pooja15ORCID,Williams Jarrod16ORCID,Li Weiqun17ORCID,Curd Matthew E.18ORCID,Burnett Timothy L.18ORCID,Robinson Ian19ORCID,Brett Dan J. L.12ORCID,Ehrhardt Matthias J.1610ORCID,Quinn Paul D.13ORCID,Mehdi Layla B.17ORCID,Withers Philip J.18ORCID,Britton Melanie M.15ORCID,Browning Nigel D.17ORCID,Shearing Paul R.12ORCID

Affiliation:

1. The Faraday Institution Quad One Harwell Science and Innovation Campus Didcot OX11 0RA UK

2. Electrochemical Innovation Lab Department of Chemical Engineering UCL London WC1E 7JE UK

3. Diamond Light Source Ltd Harwell Science and Innovation Campus Didcot OX11 0DE UK

4. Helmholtz‐Zentrum Berlin für Materialien und Energie Hahn Meitner Platz 1 14109 Berlin Germany

5. School of Chemistry University of Birmingham Birmingham B15 2TT UK

6. Department of Mathematical Sciences University of Bath Bath BA2 7AY UK

7. Department of Mechanical Materials and Aerospace Engineering University of Liverpool Liverpool L69 3GH UK

8. Henry Royce Institute Department of Materials The University of Manchester Oxford Road Manchester M13 9PL UK

9. Department of Physics and Astronomy UCL London WC1E 6BT UK

10. Institute for Mathematical Innovation University of Bath Bath BA2 7AY UK

Abstract

AbstractDemand for low carbon energy storage has highlighted the importance of imaging techniques for the characterization of electrode microstructures to determine key parameters associated with battery manufacture, operation, degradation, and failure both for next generation lithium and other novel battery systems. Here, recent progress and literature highlights from magnetic resonance, neutron, X‐ray, focused ion beam, scanning and transmission electron microscopy are summarized. Two major trends are identified: First, the use of multi‐modal microscopy in a correlative fashion, providing contrast modes spanning length‐ and time‐scales, and second, the application of machine learning to guide data collection and analysis, recognizing the role of these tools in evaluating large data streams from increasingly sophisticated imaging experiments.

Publisher

Wiley

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment

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