Surface Engineering of Binder‐free Anodes of Bi and Cu Compounds with Se and Carbon Nanotubes to Improve Lithium‐ion Batteries

Author:

Rublova Yelyzaveta1ORCID,Kong Xiangze2,Lazarenko Vitalijs1,Andzane Jana1,Meija Raimonds1,Viksna Arturs3,Kallio Tanja2,Erts Donats13

Affiliation:

1. Institute of Chemical Physics University of Latvia Raina Boulevard 19 LV-1586 Riga Latvia

2. Aalto University School of Chemical Engineering Kemistintie 1 02150 Espoo Finland

3. Faculty of Chemistry University of Latvia Raina Boulevard 19 LV-1586 Riga Latvia

Abstract

AbstractThis study focuses on the surface engineering of binder‐free anodes composed of Bi, Se, Cu, and carbon nanotubes to enhance lithium‐ion batteries. The anodes synthesized in this study showed promising electrochemical properties. However, issues with cycle stability, operational speed, and solid electrolyte interface (SEI) formation affected their overall performance. To address these challenges, the study applied different conductive polymers, namely PEO, CMC, and PEGDA‐co‐VC, to form artificial SEI layers. The application of these polymers altered the stability and efficiency of the electrodes, with the PEGDA‐co‐VC‐coated electrodes demonstrating significant stability and consistent capacity over numerous cycles.

Funder

European Regional Development Fund

Publisher

Wiley

Subject

Electrochemistry,Electrical and Electronic Engineering,Energy Engineering and Power Technology

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