Assessment of aerosol optical and physical properties and implications for radiative effects over the semiarid region of Indo‐Gangetic Basin

Abstract

This study assesses the physical and optical properties and estimated the radiative forcing of aerosol at Agra over the Indo‐Gangetic Basin (IGB) during July 2016–December 2019 using black carbon (BC) mass concentration (AE‐33 aethalometer), data sets from satellite and model simulations. The optical properties of aerosol and radiative forcing have been measured by the Optical and Physical Properties of Aerosols and Clouds (OPAC) and Santa Barbara Discrete Ordinate Radiative Transfer Atmospheric Radiative Transfer (SBDART) model. The high BC mass concentration has been observed in November and lowest in August. An adverse meteorological condition due to a combination of temperature and low wind speed results in poor dispersion in the wintertime is a common factor for high concentration level pollutants over Agra. The diurnal and temporal cycle of BC mass concentration exhibits a high concentration at nighttime due to the lower atmospheric boundary layer. The seasonal variation of absorption coefficient (βabs) and Absorption Angstrom Exponent (AAE) is found to be higher during post‐monsoon and lowest in monsoon season. This suggests that black carbon concentration over Agra is mainly generated from crop burning, waste burning, automobile exhaust and long‐range transport from Punjab and Haryana as the present site is downwind. OPAC‐derived aerosol optical depth (AOD), single‐scattering albedo (SSA), Angstrom Exponent (AE) and asymmetry parameter (AsyP) were estimated to be 0.57 ± 0.07, 0.78 ± 0.16, 0.99 ± 0.21 and 0.81 ± 0.15, respectively. AOD and AE from the OPAC and the moderate resolution imaging spectroradiometer (MODIS) have shown the consistent relationship. The mean radiative forcing is 18.3 ± 2.1 W m−2 at the top of the atmosphere while, at the surface, net radiative forcing is −42.4 ± 7.2 and 59.1 ± 6.5 W m−2 at the atmosphere during the study period. Vertical profiles were estimated using the observations from Cloud‐Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) satellite and the change in heating rate from the SBDART model over Agra.