Non‐Conductive and Conductive Washable Amylopectin‐Mastic Gum Adhesives for On‐Skin Applications

Author:

Al Boustani George12ORCID,Xu Zhuoran1,Teshima Tetsuhiko F.12,Bichlmaier Lukas3,Nikić Marta1,Hiendlmeier Lukas1,Sayn‐Wittgenstein August1,Tüzün Defne1,Inoue Shigeyoshi3,Wolfrum Bernhard12ORCID

Affiliation:

1. Neuroelectronics Munich Institute of Biomedical Engineering Department of Electrical Engineering TUM School of Computation, Information and Technology Technical University of Munich Hans‐Piloty‐Str. 1 85748 Garching Germany

2. Medical & Health Informatics Laboratories NTT Research Incorporated 940 Stewart Dr. Sunnyvale CA 94085 USA

3. TUM School of Natural Sciences Department of Chemistry Institute of Silicon Chemistry and Catalysis Research Center Technical University of Munich Lichtenbergstraße 4 85748 Garching Germany

Abstract

AbstractThe investigation of a skin adhesive based on amylopectin and mastic gum for attaching skin sensors are reported. The material provides reliable adhesion and is, at the same time, readily washable from the skin due to the hydrophilic character of the amylopectin compound. The effect of water and glycerol content on the adhesion properties in combination with polyimide‐based substrates is assessed and optimize the material for homogeneous and washable on‐skin applications. This results show that the adhesive material can withstand a shear stress of 88.7 ± 5.30 kPa in a lap shear test. The adhesive material can also be easily rendered conductive by adding sodium chloride. Impedance spectroscopy is performed on the conductive adhesive material to assess the impedance behavior during drying conditions over 24 h in comparison to commercial electrolyte gel. While the conductive adhesion material's initial impedance is slightly higher than the commercial gel, the long‐term assessment demonstrates a significantly improved stability over time. In conclusion, this study develops a skin adhesive combining amylopectin and mastic gum, demonstrating promising adhesion strength and conductivity properties, thus potentially addressing current stability challenges in skin‐sensor applications.

Funder

Bundesministerium für Bildung und Forschung

Publisher

Wiley

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