Bioinspired Gas Manipulation for Regulating Multiphase Interactions in Electrochemistry

Author:

Long Zhiyun12ORCID,Yu Cunming12ORCID,Cao Moyuan3ORCID,Ma Jun4,Jiang Lei12

Affiliation:

1. Key Laboratory of Bio‐inspired Smart Interfacial Science and Technology of Ministry of Education School of Chemistry Beihang University Beijing 100191 China

2. Key Laboratory of Bio‐inspired Materials and Interfacial Science Technical Institute of Physics and Chemistry Chinese Academy of Sciences Beijing 100190 China

3. School of Materials Science and Engineering Smart Sensing Interdisciplinary Science Center Nankai University Tianjin 300350 China

4. State Key Laboratory of Urban Water Resource and Environment Harbin Institute of Technology Harbin 150090 P. R. China

Abstract

AbstractThe manipulation of gas in multiphase interactions plays a crucial role in various electrochemical processes. Inspired by nature, researchers have explored bioinspired strategies for regulating these interactions, leading to remarkable advancements in design, mechanism, and applications. This paper provides a comprehensive overview of bioinspired gas manipulation in electrochemistry. It traces the evolution of gas manipulation in gas‐involving electrochemical reactions, highlighting the key milestones and breakthroughs achieved thus far. The paper then delves into the design principles and underlying mechanisms of superaerophobic and (super)aerophilic electrodes, as well as asymmetric electrodes. Furthermore, the applications of bioinspired gas manipulation in hydrogen evolution reaction (HER), carbon dioxide reduction reaction (CO2RR), and other gas‐involving electrochemical reactions are summarized. The promising prospects and future directions in advancing multiphase interactions through gas manipulation are also discussed.

Funder

National Key Research and Development Program of China

National Natural Science Foundation of China

China Postdoctoral Science Foundation

Publisher

Wiley

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