Highly efficient in‐situ sulfur doped graphitic carbon nitride nanoplates as an artificial photosynthetic system for NADH regeneration

Author:

Gupta Sarvesh Kumar1,Gupta Abhishek Kumar1,Yadav Rajesh Kumar2,Singh Ajeet3,Yadav B. C.3

Affiliation:

1. Nanoionics and Energy Storage Laboratory (NanoESL), Department of Physics and Material Science Madan Mohan Malaviya University of Technology Gorakhpur (U. P.) India 273010

2. Department of Chemistry and Environmental Science Madan Mohan Malaviya University of Technology Gorakhpur (U. P.) India 273010

3. Department of Physics, School of Physical & Decision Sciences, Nanomaterials and Sensors Research Laboratory Babasaheb Bhimrao Ambedkar University Lucknow (U.P)

Abstract

AbstractPhotocatalysis reduces the challenges associated with power activities by the conversion of solar energy into chemical energy. Herein, sulfur‐doped graphitic carbon nitride nanoplate (S‐g‐CN‐NP) via polycondensation and vapor oxidative treatment methods as a promising solar light‐reactive photocatalyst has been designed. The photo‐mediated reduction of NAD+ is used to facilitate the extremely efficient solar light‐driven photocatalytic selective production of nicotinamide adenine dinucleotide (NADH). The S‐g‐CN‐NP photocatalyst shown excellent optical and photoelectrical properties, supporting an NADH yield of (97±0.010 %), which was 1.5 folds higher than that of S‐g‐CN powder (65±0.012 %). Through the transformation of S‐g‐CN powder to nanoplates, the improvement of photocatalytic in S‐g‐CN‐NP was primarily ascribed to the growth of active sites of the nanoplates. The current study focuses on the creation and use of an S‐g‐CN‐NP photocatalyst for direct selective NADH regeneration under solar light.

Publisher

Wiley

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