Formation of Nucleophilic Allylboranes from Molecular Hydrogen and Allenes Catalyzed by a Pyridonate Borane that Displays Frustrated Lewis Pair Reactivity-Reference-Cited by-同舟云学术

Formation of Nucleophilic Allylboranes from Molecular Hydrogen and Allenes Catalyzed by a Pyridonate Borane that Displays Frustrated Lewis Pair Reactivity

Published:2020-10-22 Issue:52 Volume:59 Page:23885-23891
ISSN:1433-7851
Container-title:Angewandte Chemie International Edition
language:en
Short-container-title:Angew. Chem. Int. Ed.

Author:

Hasenbeck Max¹,Ahles Sebastian¹^ORCID,Averdunk Arthur¹,Becker Jonathan²,Gellrich Urs¹^ORCID

Affiliation:

1. Institut für Organische Chemie Justus-Liebig-Universität Gießen Heinrich-Buff-Ring 17 35392 Gießen Germany

2. Institut für Anorganische und Analytische Chemie Justus-Liebig-Universität Gießen Heinrich-Buff-Ring 17 35392 Gießen Germany

Funder

Verband der Chemischen Industrie

Deutsche Forschungsgemeinschaft

Publisher

Wiley

Subject

General Chemistry,Catalysis

Link

https://onlinelibrary.wiley.com/doi/pdf/10.1002/anie.202011790

Reference66 articles.

2. Asymmetric carbon-carbon bond formation via .beta.-allyldiisopinocampheylborane. Simple synthesis of secondary homoallylic alcohols with excellent enantiomeric purities

3. Chiral synthesis via organoboranes. 7. Diastereoselective and enantioselective synthesis of erythro- and threo-.beta.-methylhomoallyl alcohols via enantiomeric (Z)- and (E)-crotylboranes

4. Chiral synthesis via organoboranes. 27. Remarkably rapid and exceptionally enantioselective (approaching 100% ee) allylboration of representative aldehydes at -100.degree. under new, salt-free conditions

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