Serial Femtosecond Zero Dose Crystallography Captures a Water‐Free Distal Heme Site in a Dye‐Decolorising Peroxidase to Reveal a Catalytic Role for an Arginine in Fe IV =O Formation

Author:

Lučić Marina1ORCID,Svistunenko Dimitri A.1ORCID,Wilson Michael T.1,Chaplin Amanda K.1,Davy Bradley2,Ebrahim Ali12,Axford Danny2,Tosha Takehiko3ORCID,Sugimoto Hiroshi3ORCID,Owada Shigeki34ORCID,Dworkowski Florian S. N.5ORCID,Tews Ivo6ORCID,Owen Robin L.2,Hough Michael A.1ORCID,Worrall Jonathan A. R.1ORCID

Affiliation:

1. School of Life Sciences University of Essex Wivenhoe Park Colchester Essex CO4 3SQ UK

2. Diamond Light Source Harwell Science and Innovation Campus Didcot Oxfordshire OX11 0DE UK

3. RIKEN Spring-8 Center 1-1-1 Kouto Sayo Hyogo 679-5148 Japan

4. Japan Synchrotron Radiation Research Institute 1-1-1 Kouto Sayo Hyogo 679-5198 Japan

5. Swiss Light Source Paul Scherrer Institute 5232 Villigen PSI Switzerland

6. Biological Sciences Institute for Life Sciences University of Southampton University Road Southampton SO17 1BJ UK

Funder

Biotechnology and Biological Sciences Research Council

Publisher

Wiley

Subject

General Chemistry,Catalysis

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