Self‐Powered and Self‐Recoverable Multimodal Force Sensors Based on Trap State and Interfacial Electron Transfer

Author:

Wang Wenjie1,Tan Jie1ORCID,Wang Han1,Xiao Hua1,Shen Ruichen1,Huang Bolong2,Yuan Quan13ORCID

Affiliation:

1. Molecular Science and Biomedicine Laboratory (MBL) State Key Laboratory of Chemo/Biosensing and Chemometrics College of Chemistry and Chemical Engineering Hunan University 410082 Changsha China

2. Department of Applied Biology and Chemical Technology The Hong Kong Polytechnic University Hong Kong SAR China

3. College of Chemistry and Molecular Sciences Wuhan University 430072 Wuhan China

Abstract

AbstractMulti‐dimensional force sensing that combines intensity, location, area and the like could gather a wealth of information from mechanical stimuli. Developing materials with force‐induced optical and electrical dual responses would provide unique opportunities to multi‐dimensional force sensing, with electrical signals quantifying the force amplitude and the luminescence output providing spatial distribution of force. However, the reliance on external power supply and high‐energy excitation source brings significant challenges to the applicability of multi‐dimensional force sensors. Here we reported the mechanical energy‐driven and sunlight‐activated materials with force‐induced dual responses, and investigated the underlying mechanisms of self‐sustainable force sensing. Theoretical analysis and experimental data unraveled that trap‐controlled luminescence and interfacial electron transfer play a major role in force‐induced optical and electrical output. These materials were manufactured into pressure sensor with renewable dual‐mode output for quantifying and visualization of pressures by electrical and optical output, respectively, without power supply and high‐energy irradiation. The quantification of tactile sensation and stimuli localization of mice highlighted the multi‐dimensional sensing ability of the sensor. Overall, this self‐powered pressure sensor with multimodal output provides more modalities of force sensing, poised to change the way that intelligent devices sense with the world.

Funder

National Natural Science Foundation of China

Natural Science Foundation of Hunan Province

Publisher

Wiley

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