Optical and magneto‐optical properties of pulsed laser‐deposited thulium iron garnet thin films

Author:

Sharma Apoorva1,Ciubotariu Oana T.2,Matthes Patrick3,Okano Shun1,Zviagin Vitaly4,Kalbáčová Jana15,Gemming Sibylle67,Himcinschi Cameliu8,Grundmann Marius4,Zahn Dietrich R. T.17,Albrecht Manfred2,Salvan Georgeta17ORCID

Affiliation:

1. Semiconductor Physics, Institute of Physics Chemnitz University of Technology Chemnitz Germany

2. Institute of Physics University of Augsburg Augsburg Germany

3. Fraunhofer Institute for Electronic Nanosystems Chemnitz Germany

4. Felix‐Bloch‐Institut für Festkörperphysik Universität Leipzig Leipzig Germany

5. HORIBA Jobin Yvon GmbH Oberursel Germany

6. Theoretical Physics of Quantum Mechanical Processes and Systems, Institute of Physics Chemnitz University of Technology Chemnitz Germany

7. Center of Materials, Architectures and Integration of Nanomembranes Chemnitz University of Technology Chemnitz Germany

8. Institute of Theoretical Physics, TU Bergakademie Freiberg Freiberg Germany

Abstract

AbstractThis work presents a combined optical and magneto‐optical spectroscopic study of thulium iron garnet (Tm3Fe5O12, TmIG) films on substituted gadolinium gallium garnet (Gd2.6Ca0.4Ga4.1Mg0.25Zr0.65O12, sGGG) substrates. Spectroscopic ellipsometry, transmission spectroscopy, magneto‐optical Kerr effect spectroscopy and Raman spectroscopy results are presented for TmIG films with a thickness in the range from 20 to 300 nm grown on sGGG by pulsed laser deposition. The complex dielectric functions of TmIG and sGGG are determined and compared with previously published results for bulk yttrium iron garnet and GGG, respectively. The magneto‐optical spectroscopy corroborated with Raman spectroscopy sheds light on strain‐induced changes as a function of TmIG film thickness.

Funder

Deutsche Forschungsgemeinschaft

Publisher

Wiley

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