1. Florida State University, Department of Oceanography, Tallahassee, FL 32306, USA;
2. Present address: Georgia Institute of Technology, School of Earth and Atmospheric Sciences, Atlanta, GA 30332, USA;
3. Present address: Max-Planck Institute for Chemistry, Biogeochemistry Department D-6500 Mainz, Germany;
4. Present address: Atmospheric Environment Service, Downsview, Ontario M4H 5T4, Canada