Parametric Study of Time-Dependent Corrosion Product Activity due to56Mn,58Co, and60Co in the Primary Coolant Circuit of a Typical Pressurized Water Reactor

Author:

Rafique Muhammad12ORCID,Mirza Nasir M.3,Mirza Sikander M.3,Kearfott Kimberlee J.2,Abbasi Shahab A.1,Naeem Syed F.2

Affiliation:

1. Department of Physics, University of Azad Jammu and Kashmir, Muzaffarabad, Azad Kashmir 13100, Pakistan

2. Department of Nuclear Engineering and Radiological Sciences, University of Michigan, 2355 Bonisteel Boulevard, Ann Arbor, MI 48109-2104, USA

3. Department of Physics and Applied Mathematics, Pakistan Institute of Engineering and Applied Sciences, Nilore, Islamabad 45650, Pakistan

Abstract

Results of a detailed study, based on the parametric analysis of activated corrosion products, in primary coolant of a typical pressurized water reactor (PWR) are presented. The parameters influencing time dependent buildup of corrosion product activity (CPA) in primary coolant loop of PWR were identified. The computer program CPAIR was used to accommodate for time dependent corrosion rates. The behaviors of56Mn,58Co, and60Co were studied over the reactor operational time. During the course of normal operation of reactor, the CPA is dominated by56Mn, while58Co and60Co are the predominant radionuclides after reactor shutdown. Parametric study suggests that the total CPA is most sensitive to ion-exchanger removal rates. For a removal rate of 300 cm3-s−1, the specific activity due to56Mn has the maximum value of 3.552 × 104 Bq-m−3after 1,000 hours of reactor operation. This value decreases drastically to 8.325 × 103 Bq-m−3at removal rate of 900 cm3-s−1. Additionally, CPA due to56Mn,58Co, and60Co shows strong dependence on removal rates from the core material surfaces. Variations in the values of radionuclide removal rates from piping surface and radionuclide removal rate from deposition on pipes showed only very small effects on CPA buildup.

Funder

Higher Education Commission, Pakistan

Publisher

Hindawi Limited

Subject

General Chemistry

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