Role of Deposition Pressure on Properties of Phosphorus Doped Hydrogenated Nano-Crystalline Silicon (nc-Si:H) Thin Films Prepared by the Cat-CVD Method

Author:

Gabhale Bharat1,Waghmare Ashish1,Pandharkar Subhash1,Bhorde Ajinkya1,Nair Shruthi1,Vairale Priti1,Doiphode Vidya1,Shinde Pratibha1,Punde Ashvini1,Hase Yogesh1,Patil Nilesh1,Prasad Mohit2,Jadkar Sandesh2

Affiliation:

1. School of Energy Studies, Savitribai Phule Pune University, Pune 411 007,India

2. Department of Physics, Savitribai Phule Pune University, Pune 411 007,India

Abstract

Objective: Phosphorus doped hydrogenated nano-crystalline silicon (nc-Si:H) thin films were synthesized by catalytic chemical vapor deposition (Cat-CVD) method. Methods: The effect of deposition pressure on opto-electronic and structural properties was studied using various analysis techniques such as low angle XRD analysis, FTIR spectroscopy, Raman spectroscopy, UV-Visible spectroscopy, dark conductivity, etc. Results: From low angle XRD and Raman spectroscopy analysis, it is observed that an increase in deposition pressure causes Si:H films to transform and transit from amorphous to the crystalline phase. At optimized deposition pressure (300 mTorr), phosphorous doped nc- Si:H films having a crystallite size of ∼29 nm and crystalline volume fraction of ∼58% along with high deposition rate (∼29.7 Å/s) have been obtained. The band gap was found to be ∼1.98 eV and hydrogen content was as low as (∼1.72 at. %) for these films. Conclusion: The deposited films can be useful as an n-type layer for Si:H based p-i-n, tandem and c-Si hetero-junction solar cells.

Publisher

Bentham Science Publishers Ltd.

Subject

General Chemical Engineering

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