Gas permeability of a compacted bentonite–sand mixture: coupled effects of water content, dry density, and confining pressure

Abstract

The gas-tightness of compacted bentonite–sand mixtures is important to the total sealing efficiency of geological repositories. The initial aim of this work was to determine whether the combination of a high confining pressure (Pc) and incomplete saturation could cause a bentonite–sand mixture to become gas-tight. The results show that the physical characteristics of the materials (degree of saturation, Sr; porosity, [Formula: see text]; and dry density, ρd) are very sensitive to changes in the applied confining pressures and their own swelling deformation (or shrinkage). The combination of these changes affects the sample’s effective gas permeability (Keff). For materials prepared at a relative humidity (RH) of 98%, Keff decreased from 10−16 to 10−20 m2 when Pc increased from 1 to 7 MPa. This means that gas-tightness can be obtained for a compacted bentonite–sand mixture when the materials experience a series of changes (e.g., w, Sr, [Formula: see text], and ρd). In addition, larger irreversible deformation (or hysteresis) was observed during the loading–unloading cycle for the sample with higher water content. This phenomenon may be attributed to larger interactions between the macrostructural and microstructural deformations and the decrease of preconsolidation pressure during hydration.