Time/frequency-domain characterization of a mid-IR DFG frequency comb via two-photon and heterodyne detection

Author:

Gabbrielli Tecla1ORCID,Insero Giacomo23,De Regis Michele12,Corrias Nicola124ORCID,Galli Iacopo15,Mazzotti Davide15ORCID,Bartolini Paolo1,Hyun Huh Jeong6,Cleff Carsten6,Kastner Alexander6,Holzwarth Ronald6,Borri Simone17ORCID,Consolino Luigi1ORCID,De Natale Paolo127ORCID,Cappelli Francesco1ORCID

Affiliation:

1. LENS – European Laboratory for Non-Linear Spectroscopy

2. CNR-INO – Istituto Nazionale di Ottica

3. University of Florence

4. QTI S.r.l.

5. ppqSense S.r.l.

6. Menlo Systems GmbH

7. INFN – Istituto Nazionale di Fisica Nucleare

Abstract

Mid-infrared frequency combs are nowadays well-appreciated sources for spectroscopy and frequency metrology. Here, a comprehensive approach for characterizing a difference-frequency-generated mid-infrared frequency comb (DFG-comb) both in the time and in the frequency domain is presented. An autocorrelation scheme exploiting mid-infrared two-photon detection is used for characterizing the pulse width and to verify the optimal compression of the generated pulses reaching a pulse duration (FWHM) as low as 196 fs. A second scheme based on mid-infrared heterodyne detection employing two independent narrow-linewidth quantum cascade lasers (QCLs) is used for frequency-narrowing the modes of the DFG-comb down to 9.4 kHz on a 5-ms timescale.

Funder

European Union

QuantERA

Horizon Europe Framework Programme

Horizon 2020 Framework Programme

Italian ESFRI Roadmap

Fondazione Cassa di Risparmio di Firenze

Publisher

Optica Publishing Group

Subject

Atomic and Molecular Physics, and Optics

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