Breakdown of argon by a train of high-repetition long-wave-infrared pulses from a free-electron laser oscillator

Abstract

This study presents an experimental demonstration of laser-induced breakdown in argon, employing a free-electron laser with a wavelength of 10 μm and a repetition rate of 2.856 GHz. Despite the fluence of individual laser pulses being an order of magnitude smaller than the breakdown threshold, cascade ionization developed in the pulse train, leading to breakdown. The breakdown probability within a finite pulse train increases with gas pressure, and it was notably enhanced in a gas chamber with poor cleanliness. Numerical simulations of cascade ionization replicated the experimental results. The simulation revealed that breakdown phenomena are governed by the balance between avalanche multiplication of electrons within laser pulses and electron diffusion during pulse intervals.