Interferometric measurements of the resonant nonlinearity of IR-active minor air constituents

Author:

Pigeon J. J.1,Tochitsky S. Ya.2,Tovey D.2,Louwrens G. J.2,Ben-Zvi I.1,Joshi C.2

Affiliation:

1. Stony Brook University

2. University of California at Los Angeles

Abstract

The resonant nonlinear refractive indices of important IR-active, minor air constituents at mid-IR and long-wave IR wavelengths were measured using a Mach–Zehnder interferometer. Measurements in H 2 O vapor were performed near 2.94, 9.3, and 10.2 µm wavelengths, and measurements in C O 2 and CO gas were performed near 9.3 µm. These measurements suggest that the nonlinearity of air can be greatly increased for relatively narrowband mid-IR and long-wave IR laser pulses.

Funder

Office of Naval Research

Publisher

Optica Publishing Group

Subject

Atomic and Molecular Physics, and Optics,Statistical and Nonlinear Physics

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