Investigation of high-harmonic cutoff of metal ions driven by near-infrared laser

Abstract

The cutoff-energies of high-harmonic generation in the laser-ablated plumes of various metal targets (Ca, Mg, Fe, Zn, Ta, Mo, Al, W, In, Cu, Au, Ti, Ag) driven by near-infrared (0.8-µm) femtosecond laser are investigated and compared. Due to the low ionization potentials of metal atoms, it is believed that the observed high-harmonic cutoffs are contributed by the singly charged or even doubly charged ions. Ionization calculations using Perelomov-Popov-Terent’ev theory are performed to estimate the laser intensities at which saturation of ionization occur for different ions. Treating the calculated values as the effective driving laser intensities, the observed cutoffs from most of the targets are in reasonable agreement with the predictions of the semi-classical cutoff law.