Trapping-induced quantum beats in a van-der-Waals heterostructure microcavity observed by two-dimensional micro-spectroscopy

Author:

Li Donghai1,Shan Hangyong2,Knopf Heiko345,Watanabe Kenji6ORCID,Taniguchi Takashi6,Qin Ying7,Tongay Sefaattin7,Eilenberger Falk345,Höfling SvenORCID,Schneider Christian2,Brixner TobiasORCID

Affiliation:

1. University of Science and Technology of China

2. University of Oldenburg

3. Friedrich Schiller University

4. Fraunhofer-Institute for Applied Optics and Precision Engineering IOF

5. Max Planck School of Photonics

6. National Institute for Materials Science

7. Arizona State University

Abstract

Spatial confinement has been frequently engineered to control the flow and relaxation dynamics of exciton polaritons. While widely investigated in GaAs microcavities, exciton-polariton coupling between discretized polariton modes arising from spatially confined 2D crystals been has been less exhaustively studied. Here, we use coherent 2D photoluminescence-detected micro-spectroscopy to detect oscillating 2D peaks exclusively from a spatial trap in a microcavity with an embedded van-der-Waals heterostructure at room temperature. We observe a wide variation of oscillatory phases as a function of spectral position within the 2D spectrum, which suggests the existence of a coupling between the discretized polariton modes. The latter is accompanied by the generation of coherent phonons.

Funder

National Natural Science Foundation of China

Fundamental Research Funds for the Central Universities

European Research Council

Japan Society for the Promotion of Science

U.S. Department of Energy

Division of Electrical, Communications and Cyber Systems

Division of Materials Research

Division of Civil, Mechanical and Manufacturing Innovation

Bundesministerium für Bildung und Forschung

European Social Fund

Freistaat Thüringen

Julius-Maximilians-Universität Würzburg

Publisher

Optica Publishing Group

Subject

Electronic, Optical and Magnetic Materials

Cited by 1 articles. 订阅此论文施引文献 订阅此论文施引文献,注册后可以免费订阅5篇论文的施引文献,订阅后可以查看论文全部施引文献

1. Polaritonics: introduction to feature issue;Optical Materials Express;2023-12-13

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