Terahertz manipulation of nonlinear optical response in topological material PtBi2

Author:

Gao Y.,Zeng X. Y.12,Wang X. B.2,Shi Y. G.2,Cheng L.ORCID,Qi J.

Affiliation:

1. University of Electronic Science and Technology of China

2. Chinese Academy of Sciences

Abstract

The substantial nonlinear optical response observed in numerous topological materials renders them well-suited for optic and photonic applications, underscoring the critical need to devise effective strategies for manipulating their nonlinearity to enhance their versatility across different applications. In this Letter, we focus on the second-harmonic generation (SHG) response of the topological material PtBi2 under intense terahertz (THz) pulses and unveil the transient nonlinearity manipulated by a THz electric field. Our findings demonstrate that upon excitation of an intense THz pulse, there emerges a substantial enhancement in the SHG signal of PtBi2, which is predominantly attributed to the linear term involving the THz field, i.e., χ(2)χ(3)E THz . We also clearly observe the transient change in the nonlinear coefficients, which could arise from the excitation of the bands with linear dispersion via the intense THz pulse. These findings bear significant implications for achieving ultrafast modulation of nonlinearity in topological materials, thereby opening avenues for advanced applications in this field.

Funder

National Key Research and Development Program of China

National Natural Science Foundation of China

Guangdong Basic and Applied Basic Research Foundation

Publisher

Optica Publishing Group

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