Research on the sustainable effect of ZnS and MoS2 decorated biochar nanocomposites for removing quinolones from antibiotic-polluted aqueous solutions

Author:

Gan Ying-Jie,Wang Yue-hui,Dang Ya-ru,Hao Wen-jie,Hu Zheng-rong,Zhang Zhi-wei,Luo Yu-min,Wu Yan-bo,Song Ai-junORCID,Zhao Zhong-bao

Abstract

Antibiotic concentrations in wastewater generated by industries such as sewage treatment plants, medical pharmaceuticals and aquaculture has exceeded acceptable levels. It is particularly urgent to seek a method that can efficiently remove antibiotics. The removal potential of three quinolone antibiotics, pefloxacin (PF), levofloxacin (LF) and norfloxacin (NF), in simulated contaminated water was studied using a biochar-based nanomaterial prepared by a hydrothermal method. The data were fitted with adsorption kinetics, isotherms and thermodynamics. The results showed that ZnS–MoS2 activated biochar (ZMMBC) acheived maximum adsorption amounts of 199.42, 125.00 and 142.58 mg g–1 for PF, LF and NF, suggesting that ZMMBC has excellent adsorption performance. The adsorption mechanisms of PF, LF and NF molecules on ZMMBC include complexation, pore filling, π–π interactions, electrostatic interactions and hydrogen bond interactions.

Funder

the Talent Training Project in Hebei Province

the Hebei Normal University of Science and Technology Master's Innovation Subsidy Project in 2021

The Project of Introducing Overseas Scholars in Hebei Province

the Hebei Key Laboratory of Agroecological Safety. open project of Hebei Key Laboratory of Agroecological Safety

Publisher

CSIRO Publishing

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