Abstract
Compounds of the empirical
formula Cu(HIm)2(Im)X
[where X = NO3-,
ClO4-, Cl-, Br-, and I-; HIm =
imidazole and Im- = anion of imidazole] have been
prepared and investigated. Evidence for the imidazolato
anion acting as a bridging ligand in the solid state is based on magnetic and
spectroscopic data. The electronic spectra of aqueous solutions of tetrakisimidazolecopper(11) compounds suggest the presence
of the binuclear hydroxy-bridged cation (1) :
(See diagram in article)
which is also furnished by
the imidazolato-bridged species in aqueous solution.
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