Abstract
The thermodynamic
properties of the krypton/graphite interface have been evaluated by the grand
canonical ensemble Monte Carlo method. Submonolayer adsorption isotherms have
been calculated at temperatures of 77.31, 84.11 and 90.12 K, together with
particle distribution functions, surface pressures and isosteric
heats of adsorption. The results are compared with experiment and discussed in
relation to the existence of surface phase transitions. The Monte Carlo
adsorptions were used to check the error in assuming Henry's law adsorption at
low pressure.
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