Abstract
The nuclear quadrupole
resonance frequencies of the halogen atoms in the trihalide
ions 13 and Ibr2 in some of
their crystalline salts have been measured. The results have been correlated with a simple
LOAD-MO bonding description and the charge distributions in the ions have been
calculated. These ions can be regarded as charge-transfer complexes as
described by Mulliken. The effect of the crystal
field on the charge distribution in the I3 ion has been
investigated.
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