Quantitative Sum-Frequency Generation Vibrational Spectroscopy of Molecular Surfaces and Interfaces: Lineshape, Polarization, and Orientation-Reference-Cited by-同舟云学术

Quantitative Sum-Frequency Generation Vibrational Spectroscopy of Molecular Surfaces and Interfaces: Lineshape, Polarization, and Orientation

Published:2015-04-01 Issue:1 Volume:66 Page:189-216
ISSN:0066-426X
Container-title:Annual Review of Physical Chemistry
language:en
Short-container-title:Annu. Rev. Phys. Chem.

Author:

Wang Hong-Fei¹,Velarde Luis²,Gan Wei³,Fu Li¹

Affiliation:

1. William R. Wiley Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory, Richland, Washington 99352;

2. Department of Chemistry, University at Buffalo, The State University of New York, Buffalo, New York 14260

3. Xinjiang Technical Institute of Physics and Chemistry, Chinese Academy of Sciences, Urumqi, Xinjiang 830011, China

Abstract

Sum-frequency generation vibrational spectroscopy (SFG-VS) can provide detailed information and understanding of the molecular composition, interactions, and orientational and conformational structure of surfaces and interfaces through quantitative measurement and analysis. In this review, we present the current status of and discuss important recent developments in the measurement of intrinsic SFG spectral lineshapes and formulations for polarization measurements and orientational analysis of SFG-VS spectra. The focus of this review is to present a coherent description of SFG-VS and discuss the main concepts and issues that can help advance this technique as a quantitative analytical research tool for revealing the chemistry and physics of complex molecular surfaces and interfaces.

Publisher

Annual Reviews

Subject

Physical and Theoretical Chemistry

Link

https://www.annualreviews.org/doi/pdf/10.1146/annurev-physchem-040214-121322

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