Author:
Song Meng-Ting,Zhang Yue,Huang Wen-Juan,Hou Hua-Yi,Chen Xiang-Bai, ,
Abstract
Laser Raman spectroscopy is used to study the enhancement effect of two-magnon scattering in nickel oxide through annealing treatment in a temperature range from 450 ℃ to 1050 ℃, and investigate laser heating effect on two-magnon scattering. Our study shows that two-magnon scattering of nickel oxide can be tremendously enhanced with annealing temperature rising. In the temperature range from 450 ℃ to 1050 ℃, the enhancement increases with annealing temperature increasing, and with 1050 ℃ annealing the two-magnon scattering can be enhanced more than two orders of magnitude, also the enhancement of two-magnon scattering is much stronger than that of two-phonon scattering. This tremendous enhancement is correlated not only with the significant decrease of Ni-vacancy by high temperature annealing, but also with the magnetic spin ordering network of Ni ions. The variation of sensitive intensity of two-magnon scattering with the concentration of Ni-vacancy can be used to provide a simple Raman spectroscopy method of quantitatively measuring the Ni-vacancy in nickel oxide. In addition, the annealing treatment can significantly reduce the laser heating effect on two-magnon scatting in nickel oxide power samples. At low annealing temperature, the intensity of two-magnon scattering quickly quenches with increasing laser power. With 1050 ℃ annealing, the laser heating effect on two-magnon scattering is significantly reduced and two-magnon scattering can still have strong intensity at high laser power.
Publisher
Acta Physica Sinica, Chinese Physical Society and Institute of Physics, Chinese Academy of Sciences
Subject
General Physics and Astronomy
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