Isotopic evidence for acidity-driven enhancement of sulfate formation after SO 2 emission control

Author:

Hattori Shohei1ORCID,Iizuka Yoshinori2ORCID,Alexander Becky3ORCID,Ishino Sakiko14ORCID,Fujita Koji5ORCID,Zhai Shuting3ORCID,Sherwen Tomás67ORCID,Oshima Naga8ORCID,Uemura Ryu5ORCID,Yamada Akinori9ORCID,Suzuki Nozomi1,Matoba Sumito2ORCID,Tsuruta Asuka1,Savarino Joel10ORCID,Yoshida Naohiro11112ORCID

Affiliation:

1. Department of Chemical Science and Engineering, School of Materials and Chemical Technology, Tokyo Institute of Technology, Yokohama 226-8502, Japan.

2. Institute of Low Temperature Science, Hokkaido University, Sapporo 060-0819, Japan.

3. Department of Atmospheric Sciences, University of Washington, Seattle, WA 98195-1640, USA.

4. National Institute of Polar Research, Research Organization of Information and Systems, Tokyo 190-8518, Japan.

5. Graduate School of Environmental Studies, Nagoya University, Nagoya 464-8601, Japan.

6. National Centre for Atmospheric Science, University of York, York YO10 5DD, UK.

7. Wolfson Atmospheric Chemistry Laboratories, University of York, York YO10 5DD, UK.

8. Meteorological Research Institute, Tsukuba 305-0052, Japan.

9. Toshima Electric Ltd., Tokyo 170-0005, Japan.

10. University of Grenoble Alpes, CNRS, IRD, Grenoble INP, IGE, F-38000, Grenoble, France.

11. Earth-Life Science Institute, Tokyo Institute of Technology, Tokyo 152-8551, Japan.

12. National Institute of Information and Communications Technology, Tokyo 184-8795, Japan.

Abstract

Observed 17 O excess of ice core sulfate suggests recent changes in sulfate production pathways due to lower acidity.

Funder

NSF Office of the Director

Japan Society for the Promotion of Science

Ministry of Education, Culture, Sports, Science, and Technology

Hokkaido University

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

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