Colossal magnetoresistance in the multiple wave vector charge density wave regime of an antiferromagnetic Dirac semimetal

Author:

Singha Ratnadwip1ORCID,Dalgaard Kirstine J.1ORCID,Marchenko Dmitry2ORCID,Krivenkov Maxim2ORCID,Rienks Emile D. L.2ORCID,Jovanovic Milena1,Teicher Samuel M. L.3ORCID,Hu Jiayi4,Salters Tyger H.1ORCID,Lin Jingjing4,Varykhalov Andrei2ORCID,Ong N. Phuan4ORCID,Schoop Leslie M.1ORCID

Affiliation:

1. Department of Chemistry, Princeton University, Princeton, NJ 08544, USA.

2. Helmholtz-Zentrum Berlin f‌ür Materialien und Energie, Elektronenspeicherring BESSY II, Albert-Einstein-Straße 15, 12489 Berlin, Germany.

3. Materials Department and Materials Research Laboratory, University of California, Santa Barbara, Santa Barbara, CA. 93106, USA.

4. Department of Physics, Princeton University, Princeton, NJ 08544, USA.

Abstract

Colossal negative magnetoresistance is a well-known phenomenon, notably observed in hole-doped ferromagnetic manganites. It remains a major research topic due to its potential in technological applications. In contrast, topological semimetals show large but positive magnetoresistance, originated from the high-mobility charge carriers. Here, we show that in the highly electron-doped region, the Dirac semimetal CeSbTe demonstrates similar properties as the manganites. CeSb 0.11 Te 1.90 hosts multiple charge density wave modulation vectors and has a complex magnetic phase diagram. We confirm that this compound is an antiferromagnetic Dirac semimetal. Despite having a metallic Fermi surface, the electronic transport properties are semiconductor-like and deviate from known theoretical models. An external magnetic field induces a semiconductor metal–like transition, which results in a colossal negative magnetoresistance. Moreover, signatures of the coupling between the charge density wave and a spin modulation are observed in resistivity. This spin modulation also produces a giant anomalous Hall response.

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

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