Intrinsic 2D-XY ferromagnetism in a van der Waals monolayer

Author:

Bedoya-Pinto Amilcar1ORCID,Ji Jing-Rong1ORCID,Pandeya Avanindra K.1ORCID,Gargiani Pierluigi2ORCID,Valvidares Manuel2ORCID,Sessi Paolo1ORCID,Taylor James M.3ORCID,Radu Florin3ORCID,Chang Kai1ORCID,Parkin Stuart S. P.1ORCID

Affiliation:

1. NISE Department, Max Planck Institute of Microstructure Physics, Halle, Germany.

2. ALBA Synchrotron Light Source, Barcelona, Spain.

3. Helmholtz-Zentrum für Materialien und Energie, Berlin, Germany.

Abstract

Taking the measure of a magnet The recent discovery of magnetism in two-dimensional (2D) materials has inspired efforts to understand its nature. Whereas the magnetism of monolayers of chromium iodide (CrI 3 ) can be understood in terms of out-of-plane magnetic anisotropy, the related material chromium chloride (CrCl 3 ) has spins that lie in the plane. Bedoya-Pinto et al . used molecular beam epitaxy to grow monolayers of CrCl 3 on graphene and studied its magnetic properties. Using x-ray magnetic circular dichroism measurements, the authors found that monolayer CrCl 3 is a ferromagnet, unlike bulk CrCl 3 , which is antiferromagnetic. The scaling of the signal in the critical region indicated that the material belongs to the 2D-XY universality class, distinct from Ising magnetism, which some other 2D magnets exhibit. —JS

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

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