Attosecond dynamics through a Fano resonance: Monitoring the birth of a photoelectron

Author:

Gruson V.1,Barreau L.1,Jiménez-Galan Á.2,Risoud F.3,Caillat J.3,Maquet A.3,Carré B.1,Lepetit F.1,Hergott J.-F.1,Ruchon T.1,Argenti L.2,Taïeb R.3,Martín F.245,Salières P.1

Affiliation:

1. LIDYL, CEA, CNRS, Université Paris-Saclay, CEA Saclay, 91191 Gif-Sur-Yvette, France.

2. Departamento de Química, Módulo 13, Universidad Autónoma de Madrid, 28049 Madrid, Spain.

3. Sorbonne Université, UPMC Université Paris 6, UMR 7614, Laboratoire de Chimie Physique-Matière et Rayonnement, 75231 Paris Cedex 05, France, and CNRS, UMR 7614, LCPMR, Paris, France.

4. Instituto Madrileño de Estudios Avanzados en Nanociencia (IMDEA-Nanociencia), Cantoblanco, 28049 Madrid, Spain.

5. Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid, 28049 Madrid, Spain.

Abstract

Watching as helium goes topsy-turvy Theorists have long pondered the underpinnings of the Fano resonance, a spectral feature that resembles adjacent rightside-up and upside-down peaks. An especially well-studied instance of this feature appears in the electronic spectrum of helium as a transient state undergoes delayed ionization. Two studies have now traced the dynamics of this state in real time. Gruson et al. used photoelectron spectroscopy to extract the amplitude and phase of the electron wave packet after inducing its interference with reference wave packets tuned into resonance at variable delays. Kaldun et al. used extreme ultraviolet absorption spectroscopy to probe the transient state while variably forcing ionization with a strong near-infrared field. Science , this issue pp. 734 and 738

Funder

European Union

Agence Nationale de la Recherche

European Research Council

European COST Action

MINECO

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

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