Affiliation:
1. Department of Geosciences and the EMS Environment Institute, Pennsylvania State University, UniversityPark, PA 16802, USA.
Abstract
Paleoatmospheric records of trace-gas concentrations recovered from ice cores provide important sources of information on many biogeochemical cycles involving carbon, nitrogen, and oxygen. Here, we present a 106,000-year record of atmospheric nitrous oxide (N
2
O) along with corresponding isotopic records spanning the last 30,000 years, which together suggest minimal changes in the ratio of marine to terrestrial N
2
O production. During the last glacial termination, both marine and oceanic N
2
O emissions increased by 40 ± 8%. We speculate that our records do not support those hypotheses that invoke enhanced export production to explain low carbon dioxide values during glacial periods.
Publisher
American Association for the Advancement of Science (AAAS)
Reference47 articles.
1. Current N 2 O emissions from the terrestrial biosphere are estimated to be 12 ± 3 Tg N/year and preanthropogenic estimates are ∼7 Tg N/year ( 12 36-39 ). Marine N 2 O emissions are estimated to be 4 ± 2 Tg N/year ( 40 41 ). About 98% of the total atmospheric N 2 O sink occurs in the stratosphere. Minschwaner et al. ( 42 ) estimated the 1980 value to be 12 ± 4 Tg N/year corresponding to a mean atmospheric lifetime of 118 ± 25 years ( 43 ).
2. J. R. Holton et al., Rev. Geophys.33, 403 (1995).
3. Variations in Atmospheric N
2
O Concentration During Abrupt Climatic Changes
4. J. Fluckiger et al., Global Biogeochem. Cycles16, 1010, doi:10.1029/2001GB001417 (2002).
5. M. Leuenberger, U. Siegenthaler, Nature360, 449 (1992).
Cited by
141 articles.
订阅此论文施引文献
订阅此论文施引文献,注册后可以免费订阅5篇论文的施引文献,订阅后可以查看论文全部施引文献