Femtosecond Phase-Coherent Two-Dimensional Spectroscopy-Reference-Cited by-同舟云学术

Femtosecond Phase-Coherent Two-Dimensional Spectroscopy

Published:2003-06-06 Issue:5625 Volume:300 Page:1553-1555
ISSN:0036-8075
Container-title:Science
language:en
Short-container-title:Science

Author:

Tian Peifang¹²³,Keusters Dorine¹²³,Suzaki Yoshifumi¹²³,Warren Warren S.¹²³

Affiliation:

1. Department of Electrical Engineering, Center of Ultrafast Laser Applications, Princeton University, Princeton, NJ 08544, USA.

2. Department of Chemistry, Center of Ultrafast Laser Applications, Princeton University, Princeton, NJ 08544, USA.

3. Department of Advanced Materials Science, Faculty of Engineering, Kagawa University, Takamatsu, Kagawa 761–0396, Japan.

Abstract

Femtosecond phase-coherent two-dimensional (2D) spectroscopy has been experimentally demonstrated as the direct optical analog of 2D nuclear magnetic resonance. An acousto-optic pulse shaper created a collinear three-pulse sequence with well-controlled and variable interpulse delays and phases,which interacted with a model atomic system of rubidium vapor. The desired nonlinear polarization was selected by phase cycling (coadding experimental results obtained with different interpulse phases). This method may enhance our ability to probe the femtosecond structural dynamics of macromolecules.

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

Reference27 articles.

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2. Principles of Nuclear Magnetic Resonance in One and Two Dimensions 1987

3. Preface

4. Two-dimensional Fourier transform electronic spectroscopy

5. Two-dimensional infrared spectroscopy of peptides by phase-controlled femtosecond vibrational photon echoes

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