Highly Polarized Photoluminescence and Photodetection from Single Indium Phosphide Nanowires

Author:

Wang Jianfang1,Gudiksen Mark S.1,Duan Xiangfeng1,Cui Yi1,Lieber Charles M.12

Affiliation:

1. Department of Chemistry and Chemical Biology,

2. Division of Engineering and Applied Sciences, Harvard University, Cambridge, MA 02138, USA.

Abstract

We have characterized the fundamental photoluminescence (PL) properties of individual, isolated indium phosphide (InP) nanowires to define their potential for optoelectronics. Polarization-sensitive measurements reveal a striking anisotropy in the PL intensity recorded parallel and perpendicular to the long axis of a nanowire. The order-of-magnitude polarization anisotropy was quantitatively explained in terms of the large dielectric contrast between these free-standing nanowires and surrounding environment, as opposed to quantum confinement effects. This intrinsic anisotropy was used to create polarization-sensitive nanoscale photodetectors that may prove useful in integrated photonic circuits, optical switches and interconnects, near-field imaging, and high-resolution detectors.

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

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