Interface engineering for high-performance, triple-halide perovskite–silicon tandem solar cells-Reference-Cited by-同舟云学术

Interface engineering for high-performance, triple-halide perovskite–silicon tandem solar cells

Published:2023-07-07 Issue:6653 Volume:381 Page:63-69
ISSN:0036-8075
Container-title:Science
language:en
Short-container-title:Science

Author:

Mariotti Silvia¹^ORCID,Köhnen Eike¹^ORCID,Scheler Florian¹^ORCID,Sveinbjörnsson Kári¹^ORCID,Zimmermann Lea¹^ORCID,Piot Manuel¹²^ORCID,Yang Fengjiu¹^ORCID,Li Bor¹^ORCID,Warby Jonathan³,Musiienko Artem¹^ORCID,Menzel Dorothee¹^ORCID,Lang Felix³^ORCID,Keßler Sebastian¹^ORCID,Levine Igal¹^ORCID,Mantione Daniele⁴⁵⁶^ORCID,Al-Ashouri Amran¹^ORCID,Härtel Marlene S.¹^ORCID,Xu Ke¹,Cruz Alexandros¹^ORCID,Kurpiers Jona¹^ORCID,Wagner Philipp¹^ORCID,Köbler Hans¹^ORCID,Li Jinzhao¹,Magomedov Artiom⁷^ORCID,Mecerreyes David⁴⁶,Unger Eva¹^ORCID,Abate Antonio¹^ORCID,Stolterfoht Martin³^ORCID,Stannowski Bernd¹^ORCID,Schlatmann Rutger¹^ORCID,Korte Lars¹^ORCID,Albrecht Steve¹⁸^ORCID

Affiliation:

1. Solar Energy Division, Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, 12489 Berlin, Germany.

2. Laboratory of Semiconductor Materials, Institute of Materials, Faculty of Engineering, Ecole Polytechnique Fédérale de Lausanne, 1015 Lausanne, Switzerland.

3. Institute of Physics and Astronomy, University of Potsdam, 14476 Potsdam, Germany.

4. POLYKEY Polymers, Joxe Mari Korta Center, 20018 Donostia-San Sebastian, Spain.

5. POLYMAT, University of the Basque Country UPV/EHU, 20018 Donostia-San Sebastián, Spain.

6. IKERBASQUE, Basque Foundation for Science, 48009 Bilbao, Spain.

7. Kaunas University of Technology, Kaunas, Lithuania.

8. Technische Universität Berlin, Fakultät Elektrotechnik und Informatik, 10587 Berlin, Germany.

Abstract

Improved stability and efficiency of two-terminal monolithic perovskite-silicon tandem solar cells will require reductions in recombination losses. By combining a triple-halide perovskite (1.68 electron volt bandgap) with a piperazinium iodide interfacial modification, we improved the band alignment, reduced nonradiative recombination losses, and enhanced charge extraction at the electron-selective contact. Solar cells showed open-circuit voltages of up to 1.28 volts in p-i-n single junctions and 2.00 volts in perovskite-silicon tandem solar cells. The tandem cells achieve certified power conversion efficiencies of up to 32.5%.

Publisher

American Association for the Advancement of Science (AAAS)

Subject

Multidisciplinary

Link

https://www.science.org/doi/pdf/10.1126/science.adf5872

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