Mercury (Hg) in Ryugu particles and implications for the origin of volatile elements in early Earth

Author:

Shirai Naoki1ORCID,Ito Motoo2ORCID,Yamaguchi Akira3ORCID,Tomioka Naotaka2ORCID,Uesugi Masayuki4ORCID,Imae Naoya3,Kimura Makoto3ORCID,Greenwood Richard5ORCID,Liu Ming-Chang6ORCID,Ohigashi Takuji7ORCID,Sekimoto Shun8,Uesugi Kentaro4ORCID,Nakato Aiko3ORCID,Yogata Kasumi9ORCID,Yuzawa Hayato10ORCID,Kodama Yu11,Hirahara Kaori12ORCID,Sakurai Ikuya13ORCID,Okada Ikuo13,Karouji Yuzuru12ORCID,Nakazawa Satoru14ORCID,Okada Tatsuaki14ORCID,Tanaka Satoshi9,Saiki Takanao14,Terui Fuyuto15,Yoshikawa Makoto14,Miyazaki Akiko9ORCID,Nishimura Masahiro9,Yada Toru14ORCID,Abe Masanao14,Usui Tomohiro9ORCID,Watanabe Sei-ichiro13ORCID,Tsuda Yuichi14

Affiliation:

1. Kanagawa University

2. Japan Agency for Marine-Earth Science and Technology

3. National Institute of Polar Research

4. Japan Synchrotron Radiation Research Institute

5. The Open University

6. Lawrence Livermore National Laboratory

7. Photon Factory/Institute of Materials Science, High Energy Accelerator Research Organization

8. Kyoto University

9. JAXA

10. Institute for Molecular Science, UVSOR Synchrotron Facility

11. Marine Works Japan, Ltd

12. Osaka University

13. Nagoya University

14. Japan Aerospace Exploration Agency

15. Kanagawa Institute of Technology

Abstract

Abstract

Solar system abundances of the elements, which are determined by spectroscopic measurements of the solar photosphere and laboratory analyses of CI (Ivuna-type) carbonaceous chondrites, are a cornerstone to understand the origin and evolution of planets and other constituents, such as asteroids and comets. Mercury (Hg) is one of the elements whose solar system abundance is still poorly constrained due to no observable lines for Hg in the solar spectrum and large variations of the Hg abundance in CI chondrites caused by mainly terrestrial contamination. Here we determined elemental abundances including Hg for uncontaminated CI-like material from asteroid Ryugu by the Hayabusa2 spacecraft. The new solar system abundance of Hg is 0.907±0.108 atoms/106 Si atoms. Our results demonstrate that Hg in bulk silicate Earth originated from the addition of chondritic material after core formation, late sulfide segregation and/or degassing, and volatile elements are depleted in late-accreted materials relative to CI chondrites.

Publisher

Research Square Platform LLC

Reference50 articles.

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