M2 Macrophage-Polarized Anti-inflammatory Microneedle Patch for Accelerating Biofilm-Infected Diabetic Wound Healing via Modulating the Insulin Pathway

Author:

Yang Yushan1,Fan Limin1,Jiang Jingsi2,Sun Jiuyuan1,Xue Liangyi1,Ma Xiaoyi1,Kuai Le3,Li Bin4,Li Yong Yong1

Affiliation:

1. Tongji University School of Medicine

2. Shanghai Skin Disease Hospital of Tongji University, Tongji University

3. Shanghai University of Traditional Chinese Medicine

4. Shanghai Skin Disease Hospital of Tongji University

Abstract

Abstract

Macrophages play a pivotal role in the healing of diabetic ulcers. The sustained elevation of glucose levels damages the insulin signaling pathway in macrophages, leading to dysfunctional macrophages that struggle to transition from pro-inflammatory (M1) to reparative (M2) states. Therefore, modulating macrophage inflammatory responses via the insulin pathway holds promise for diabetic ulcer treatment. Additionally, the presence of biofilm impedes drug penetration, and the resulting immunosuppressive microenvironment exacerbates the persistent infiltration of pro-inflammatory M1 macrophages. Therefore, we designed an array of dissolvable microneedle (denoted as NPF@MN) loaded with self-assembled nanoparticles that could disrupt mature biofilm structures to deliver NPF nanoparticles, acid-sensitive NPF-releasing Protocatechualdehyde (PA) with hypoglycemic and insulin-like effects, regulating macrophage polarization to an anti-inflammatory M2 phenotype. Additionally, this study extensively examined the mechanism by which NPF@MN accelerates the healing of diabetic ulcers through the activation of the insulin signaling pathway. Through RNA-seq and GSEA analysis, we identified a reduction in the expression of pathway-related factors such as IR, IRS-1, IRS-2, and SHC. Our work presents an innovative therapeutic approach targeting the insulin pathway in diabetic ulcers and underscores its translational potential for clinical management.

Publisher

Springer Science and Business Media LLC

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