Utilization of different radionuclides for high-energy extended efficiency calibration of HPGe for improved determination of calcium and sulfur using k0-INAA

Author:

Soliman Mohamed Ali1ORCID,Mindil Ahmed2,Takamiya Koichi3

Affiliation:

1. Egyptian Atomic Energy Authority

2. University of Jeddah

3. Kyoto University: Kyoto Daigaku

Abstract

Abstract The present study reports on the performance of three reactor-produced radionuclides (24Na, 56Mn, and 72Ga) and one accelerator-produced radionuclide (56Co) for extending the full energy peak efficiency calibration of a coaxial HPGe detector up to ~3100 keV at different detector to source distance. The differences in the efficiency curves obtained with and without the use of high-energy gamma emitters radionuclides have a considerable impact on the accuracy of Na, Ca, and S determination by the k0-INAA as evidenced by analysis results of reference materials. The results revealed that the use of 24Na is the most suitable radionuclide for high-energy efficiency calibration due to its reasonable availability, low production cost, simple decay scheme, and well-defined decay properties.

Publisher

Research Square Platform LLC

Reference17 articles.

1. Improvement of the Ca determination accuracy with k0-INAA using an HPGe coaxial detector with extended energy range efficiency calibration;Kučera J;J Radioannal Nucl Chem,2018

2. Wide energy range calibration method for Ge detectors;Molnar GL;Nucl Instrum Methods A,2002

3. High-energy calibration data for k0-neutron activation analysis;Szentmiklosi L;J Radioanal Nucl Chem,2018

4. IAEA (2007) Update of X-ray and gamma-ray decay data standards for detector calibration and other applications, Volume 1: Recommended decay data, high-energy gamma-ray standards and angular correlation coefficients. IAEA Vienna

5. Measurement of neutron flux parameters for implementation of k0–INAA at Kyoto University Research Reactor;Soliman MA;J Radioanal Nucl Chem,2022

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