Hydrogen storage in complex hydrides: past activities and new trends

Author:

Dematteis Erika MichelaORCID,Amdisen Mads BORCID,Autrey TomORCID,Barale JussaraORCID,Bowden Mark EORCID,Buckley Craig EORCID,Cho Young WhanORCID,Deledda Stefano,Dornheim MartinORCID,de Jongh PetraORCID,Grinderslev Jakob BORCID,Gizer GökhanORCID,Gulino ValerioORCID,Hauback Bjørn CORCID,Heere MichaelORCID,Heo Tae WookORCID,Humphries Terry DORCID,Jensen Torben RORCID,Kang Shin YoungORCID,Lee Young-SuORCID,Li Hai-WenORCID,Li SichiORCID,Møller Kasper TORCID,Ngene PeterORCID,Orimo Shin-ichiORCID,Paskevicius MarkORCID,Polanski MarekORCID,Takagi ShigeyukiORCID,Wan LiwenORCID,Wood Brandon CORCID,Hirscher MichaelORCID,Baricco MarcelloORCID

Abstract

Abstract Intense literature and research efforts have focussed on the exploration of complex hydrides for energy storage applications over the past decades. A focus was dedicated to the determination of their thermodynamic and hydrogen storage properties, due to their high gravimetric and volumetric hydrogen storage capacities, but their application has been limited because of harsh working conditions for reversible hydrogen release and uptake. The present review aims at appraising the recent advances on different complex hydride systems, coming from the proficient collaborative activities in the past years from the research groups led by the experts of the Task 40 ‘Energy Storage and Conversion Based on Hydrogen’ of the Hydrogen Technology Collaboration Programme of the International Energy Agency. An overview of materials design, synthesis, tailoring and modelling approaches, hydrogen release and uptake mechanisms and thermodynamic aspects are reviewed to define new trends and suggest new possible applications for these highly tuneable materials.

Funder

Independent research fund Denmark for technology and production

Hydrogen Technology Collaboration Programme

Hydrogen Materials-Advanced Research Consortium

Danish Ministry of Higher Education and Science

Carlsbergfondet

Australian Research Council

U.S. Department of Energy

Nederlandse Organisatie voor Wetenschappelijk Onderzoek

National Research Foundation of Korea

JSPS KAKENHI

Publisher

IOP Publishing

Subject

General Earth and Planetary Sciences,General Environmental Science

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